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You would need to encode the avi to vcd!
Try opening the file in TMPGEnc.
When you open TMPGEnc, you will get the wizard, you can use this to easily make this. Just choose vcd (pal for europe, ntsc for america). When they ask for the video & audio source, just click browse on the video source and it will automatically load the audio from it.
Click next, and click other settings. Change motion search precision to Highest Quality.
Click next a few more times and TMPGEnc will start encoding.
When its finished, it will be bigger than 800mb so click file - mpeg tools. Click merge and cut.
Click add and browse for the movies you just created with TMPGEnc. When it loads in, select it and click edit. You will see two buttons "{" and "}". Basically mean start and end.
Drag the slider accross to around 80min and click }. Now click OK. Change the file type at the top to Video CD. Now browse for somewhere to put the output 1st split of the file. Click Run.
Now when thats done, thats the movie you will have on the first cd. Click edit again. This time, click the { button where you left off last time. Now drag the slider right to the very end and click the } button.
Click ok - browse for a source to place the output 2nd split. This will be your second cd.
You now need cd writing software. I will assume Nero Burning Rom.
http://www.nero.com .
When nero loads, you will either get a new compilation window or a wizard. If you get the wizard click close wizard. Now the window will open with loads of different cd types listed on the left.
Choose Video CD and click new. You will see the vcd compilation window and a file browser. Use the file browser to find the first movie and drag it to the compilation. Click file - write cd. Repeat the step to create the second cd.